The GetSimple CMS Extend repository is an amazing collection of useful plugins and great looking themes for GetSimple. It didn't take me long to find the theme I wanted, which was a Twitter Bootstrap based theme. Unfortunately it was based on the old 2.x branch, and I couldn't find anybody who had created a theme based on the 3.x branch yet, so I decided to create my own!
You can download it from the Extend repository here: Bootstrap3 on the Extend repository
It's also available on GitHub here: Bootstrap3 on GitHub
And here's the demo: bootstrap3.randm.ca demo site
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